Portsmouth is an awesome small city. Lots of good restaurants and shops. I've done a ride that goes from Portsmouth to York Beach, Maine a couple of times. You can ride by the ocean (all 18 miles of NH coastline) and then head inland, where there's rolling hills and farms.
I'd also suggest the Camden area of Maine. Challenging riding, hiking, etc.



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but that means we'll get to bring our touring bikes for riding around on the park's carriage roads. I've only kayaked a few times, and DH never. How experienced do you need to be to kayak safely there? Are you aware of any guided excursions? I think that would be a need change of pace from our usual hiking/biking. 